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• W2953109713 startingPage "5866" @default.
• W2953109713 abstract "Highly diastereo- and enantioselective additions of substituted alpha-nitroesters to imines have been developed. High diastereoselection relies on the finding that the combination of chiral proton catalyst 2b and alpha-nitro aryl esters bearing 2,6-disubstitution combine to raise substrate-controlled diastereoselection to >20:1 in favor of the syn diastereomer. Furthermore, the chiral catalyst provides enantioselection to the 99% level through control of the addition step in which the azomethine pi-faces are differentiated. The bifunctional chiral protic acid catalyst enables these reactions to proceed without separate preactivation of either substrate, leading to a straightforward synthetic protocol for the formation of alpha,beta-diamino phenyl alanine derivatives." @default.
• W2953109713 created "2019-06-27" @default.
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• W2953109713 creator A5042662638 @default.
• W2953109713 date "2008-04-15" @default.
• W2953109713 modified "2023-09-25" @default.
• W2953109713 title "A Diastereo- and Enantioselective Synthesis of α-Substituted <i>syn</i>-α,β-Diamino Acids" @default.
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• W2953109713 doi "https://doi.org/10.1021/ja8011808" @default.
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• W2953109713 hasPublicationYear "2008" @default.
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