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• W2953301623 abstract "Abstract α‐Alkylidene cyclic carbonates (αCCs) recently emerged as attractive CO 2 ‐sourced synthons for the construction of complex organic molecules. Herein, we report the transformation of αCCs into novel families of sulfur‐containing compounds by organocatalyzed chemoselective addition of thiols, following a domino process that is switched on/off depending on the desired product. The process is extremely fast and versatile in substrate scope, provides selectively linear thiocarbonates or elusive tetrasubstituted ethylene carbonates with high yields following a 100 % atom economy reaction, and valorizes CO 2 as a renewable feedstock. It is also exploited to produce a large diversity of unprecedented functional polymers. It constitutes a robust platform for the design of new sulfur‐containing organic synthons and important families of polymers." @default.
• W2953301623 created "2019-06-27" @default.
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• W2953301623 date "2019-07-18" @default.
• W2953301623 modified "2023-10-16" @default.
• W2953301623 title "A Switchable Domino Process for the Construction of Novel CO ₂ ‐Sourced Sulfur‐Containing Building Blocks and Polymers" @default.
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• W2953301623 doi "https://doi.org/10.1002/anie.201905969" @default.
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