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- W2954121723 abstract "Electrochemical reduction of CO2 is a value-added approach to both decrease the atmospheric emission of carbon dioxide and form valuable chemicals. We present a zero gap electrolyzer cell, which continuously converts gas phase CO2 to products without using any liquid catholyte. This is the first report of a multilayer CO2 electrolyzer stack for scaling up the electrolysis process. CO formation with partial current densities above 250 mA cm-2 were achieved routinely, which was further increased to 300 mA cm-2 (with ∼95% faradic efficiency) by pressurizing the CO2 inlet (up to 10 bar). Evenly distributing the CO2 gas among the layers, the electrolyzer operates identically to the sum of multiple single-layer electrolyzer cells. When passing the CO2 gas through the layers consecutively, the CO2 conversion efficiency increased. The electrolyzer simultaneously provides high partial current density, low cell voltage (-3.0 V), high conversion efficiency (up to 40%), and high selectivity for CO production." @default.
- W2954121723 created "2019-07-12" @default.
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- W2954121723 date "2019-06-27" @default.
- W2954121723 modified "2023-10-16" @default.
- W2954121723 title "Multilayer Electrolyzer Stack Converts Carbon Dioxide to Gas Products at High Pressure with High Efficiency" @default.
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- W2954121723 doi "https://doi.org/10.1021/acsenergylett.9b01142" @default.
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