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• W2955007060 abstract "Abstract Nitrogen-doped porous carbons were prepared via chemical activation of chitosan using alkali-metal carbonates (Na2CO3, K2CO3, Rb2CO3, and Cs2CO3), and the water adsorption isotherms of prepared carbons were measured to estimate the performance of the carbons in adsorption heat pump/desiccant cooling. Pre-doping of an alkali carbonate activator into the chitosan precursor resulted in a highly developed micropore structure and the introduction of macropores. The macropore structure clearly depended on the alkali carbonate activator. Na2CO3 resulted in two-dimensional macropores because of the hard-template effect, whereas the other alkali carbonate activators resulted in three-dimensional macropores with different cell sizes. A density functional theory calculation study based on X-ray photoelectron spectroscopy analyses of nitrogen-doped activated carbons indicated that pyridinic (pyridine, pyridone, and pyridine N-oxide), amide, and quaternary N groups might be effective for low-pressure water adsorption. Although the water adsorption capacities of the prepared carbons at P/P0 > 0.5 increased with increasing micropore volume, those at the low-pressure region (P/P0" @default.
• W2955007060 created "2019-07-12" @default.
• W2955007060 creator A5006536628 @default.
• W2955007060 creator A5086240459 @default.
• W2955007060 date "2019-10-01" @default.
• W2955007060 modified "2023-09-24" @default.
• W2955007060 title "Water adsorption on nitrogen-doped carbons for adsorption heat pump/desiccant cooling: Experimental and density functional theory calculation studies" @default.
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• W2955007060 doi "https://doi.org/10.1016/j.apsusc.2019.06.267" @default.
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