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- W295560982 abstract "CH{sub 3}F, CH{sub 3}Cl, CH{sub 3}Br were seeded into Ar van der Waals clusters by means of a pulsed supersonic molecular beam. Ions formed by electron impact were observed by time-of-flight mass spectroscopy. Enhancement of the CH{sub 2}X{sup +} signal relative to the CH{sub 3}X{sup +} was noted. By changing the seed concentration it was shown that this was due to Ar rather than the (CH{sub 3}X){sub 2} dimer. These results are energetically compatible with a Penning energy transfer from Ar. Protonation of the CH{sub 3}X ions was observed related to the number of clusters containing more than one seed molecule. A difference in CH{sub 4}Cl{sup +}and CH{sub 4}Br{sup +} production was noted. This is interesting considering the similarity of the gas-phase proton affinity of the CH{sub 3}Cl and CH{sub 3}Br." @default.
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- W295560982 date "1993-05-01" @default.
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- W295560982 title "Ionization, fragmentation and protonation of CH{sub 3}X in Argon clusters under electron impact (X=F,Cl,Br)." @default.
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