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• W2955756768 abstract "Abstract Spinodal decomposition, the spontaneous phase separation process of periodic lamellae at the nanometer scale, of correlated oxide ((Ti, V)O 2 ) systems offers a sophisticated route to achieve a new class of mesoscale structures in the form of self-assembled superlattices for possible applications using steep metal–insulator transitions. Here, we achieve the tunable self-assembly of (Ti, V)O 2 superlattices with steep transitions (Δ T MI < 5 K) by spinodal decomposition with accurate control of the growth parameters without conventional layer-by-layer growth. Abrupt compositional modulation with alternating Ti-rich and V-rich layers spontaneously occurs along the growth direction because in-plane lattice mismatch is smaller in this direction than in other directions. An increase in the film growth rate thickens periodic alternating lamellae; the phase separation can be kinetically enhanced by adatom impingement during two-dimensional growth, demonstrating that the interplay between mass transport and uphill diffusion yields highly periodic (Ti, V)O 2 superlattices with tunable lamellar periods. Our results for creating correlated (Ti, V)O 2 oxide superlattices provide a new bottom-up strategy to design rutile oxide tunable nanostructures and present opportunities to design new material platforms for electronic and photonic applications with correlated oxide systems." @default.
• W2955756768 created "2019-07-12" @default.
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• W2955756768 date "2019-06-28" @default.
• W2955756768 modified "2023-10-17" @default.
• W2955756768 title "Self-assembly of correlated (Ti, V)O2 superlattices with tunable lamella periods by kinetically enhanced spinodal decomposition" @default.
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• W2955756768 doi "https://doi.org/10.1038/s41427-019-0132-z" @default.
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