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• W2955931896 abstract "The integration of molecular catalysts with low-cost, solid light absorbers presents a promising strategy to construct catalysts for the generation of solar fuels. Here, we report a photocatalyst for CO2 reduction that consists of a polymeric cobalt phthalocyanine catalyst (CoPPc) coupled with mesoporous carbon nitride (mpg-CNx) as the photosensitizer. This precious-metal-free hybrid catalyst selectively converts CO2 to CO in organic solvents under UV/Vis light (AM 1.5G, 100 mW cm−2, λ>300 nm) with a cobalt-based turnover number of 90 for CO after 60 h. Notably, the photocatalyst retains 60 % CO evolution activity under visible light irradiation (λ>400 nm) and displays moderate water tolerance. The in situ polymerization of the phthalocyanine allows control of catalyst loading and is key for achieving photocatalytic CO2 conversion." @default.
• W2955931896 created "2019-07-12" @default.
• W2955931896 creator A5019861460 @default.
• W2955931896 creator A5026491082 @default.
• W2955931896 date "2019-07-30" @default.
• W2955931896 modified "2023-10-16" @default.
• W2955931896 title "Visible‐Light‐Driven CO ₂ Reduction by Mesoporous Carbon Nitride Modified with Polymeric Cobalt Phthalocyanine" @default.
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• W2955931896 doi "https://doi.org/10.1002/ange.201907082" @default.
• W2955931896 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6771752" @default.
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• W2955931896 hasPublicationYear "2019" @default.
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