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• W2956043296 startingPage "7542" @default.
• W2956043296 abstract "High-valent iron-oxo complexes are key intermediates in C-H functionalization reactions. Herein, we report the generation of a (TAML)Fe-oxo species (TAML = tetraamido macrocyclic ligand) via electrochemical proton-coupled oxidation of the corresponding (TAML)FeIII-OH2 complex. Cyclic voltammetry (CV) and spectroelectrochemical studies are used to elucidate the relevant (TAML)Fe redox processes and determine the predominant (TAML)Fe species present in solution during bulk electrolysis. Evidence for iron(iv) and iron(v) species is presented, and these species are used in the electrochemical oxygenation of benzylic C-H bonds and dehydrogenation of alcohols to ketones." @default.
• W2956043296 created "2019-07-12" @default.
• W2956043296 creator A5047440637 @default.
• W2956043296 creator A5055963116 @default.
• W2956043296 creator A5074617275 @default.
• W2956043296 date "2019-01-01" @default.
• W2956043296 modified "2023-10-13" @default.
• W2956043296 title "Electrochemical C–H oxygenation and alcohol dehydrogenation involving Fe-oxo species using water as the oxygen source" @default.
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• W2956043296 doi "https://doi.org/10.1039/c9sc02609f" @default.
• W2956043296 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6761876" @default.
• W2956043296 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31588305" @default.
• W2956043296 hasPublicationYear "2019" @default.
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