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- W2956101407 abstract "UiO-66-NH2, as typical visible light responsive Zr-based metal-organic frameworks (MOFs), has attracted great interest in recent years. However, rapid combination of the photoinduced carriers limits its further application. Here, we designed a facile precipitation-photoreduction method to post-synthetically decorate Ag/AgCl on the surface of UiO-66-NH2 and form a heterostructure. Metallic Ag can not only transmit electrons between UiO-66-NH2 and AgCl but also absorb visible light, because of the surface plasmon resonance (SPR) effect. The rhodamine B photodegradation rate of UiO-66-NH2/Ag/AgCl (16.2 wt.% Ag) is about 10 and 4 times those of UiO-66-NH2 and Ag/AgCl, respectively. The SPR effect of Ag NPs and the formation of a heterostructure synergistically increase the absorbability of visible light, accelerate the separation of photoinduced charges, and promote the formation of superoxide radicals. We expect that our work could provide a new viewpoint for constructing efficient MOF-based photocatalytic systems." @default.
- W2956101407 created "2019-07-12" @default.
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- W2956101407 date "2019-08-01" @default.
- W2956101407 modified "2023-09-29" @default.
- W2956101407 title "Decorating Ag/AgCl on UiO-66-NH2: Synergy between Ag plasmons and heterostructure for the realization of efficient visible light photocatalysis" @default.
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- W2956101407 doi "https://doi.org/10.1016/s1872-2067(19)63377-2" @default.
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