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• W2956132008 abstract "Phase transition can profoundly influence the electrochemical performances of cathode materials for lithium ion batteries. The intricate phase transitions upon electrochemical cycling constrain the high-rate performances of the LiNi₀.₅Mn₁.₅O₄ cathode. The formation of the rocksalt-like phase causes the diffusion of Li ions asymmetric in the lithiation and delithiation reactions. The evolution of multiple cubic phases results in poor diffusivity of Li ions in the LiNi₀.₅Mn₁.₅O₄. High-resolution XRD scans on the chemically delithiated samples reveal that the intricate phase transitions are effectively suppressed in Cr-doped LiNi₀.₅Mn₁.₅O₄. The suppression of phase transitions not only enhances the Li ions’ diffusivity inside the lattice, but also stabilizes the charge transfer interfaces by reducing lattice mismatch and alleviating structural stress during the lithiation and delithiation. Consequently, the improvement on structure evolution endows the LiNi₀.₅Mn₁.₅O₄ with enhanced diffusion coefficient of Li ions, larger accessible capacity, and improved Coulombic efficiency." @default.
• W2956132008 created "2019-07-12" @default.
• W2956132008 creator A5000159653 @default.
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• W2956132008 date "2018-01-01" @default.
• W2956132008 modified "2023-09-24" @default.
• W2956132008 title "Phase Transition Dominated High-Rate Performances of the High Voltage LiNi₀.₅Mn₁.₅O₄ Cathode: Improvement on Structure Evolution and Ionic Diffusivity by Chromium Doping" @default.
• W2956132008 hasPublicationYear "2018" @default.
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