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- W2956161692 abstract "The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behavior, here we describe a system in which the structural disorder destroys a disordered moment fragmentation system resulting in long-range antiferromagnetic order due to local symmetry breaking. Nd$_2$ScNbO$_7$ is shown to have traces of moment fragmentation behavior through polarized and inelastic neutron scattering. However this is shown to only occur on 14.0(2) % of the neodymium ions. The remaining magnetic species order completely into the all-in all-out Ising antiferromagnetic structure. This can be seen as a result of local symmetry breaking due disordered Sc$^{+3}$ and Nb$^{+5}$ ions about the A-site. As the moment fragmentation phenomenon is closely linked to the $overline{D_{3d}}$ symmetry, it is proposed that only systems retaining this symmetry, or the reduced $overline{D_3}$ symmetry exhibit moment fragmentation. However, the phenomenon of moment fragmentation in magnetic pyrochlore lattices is very robust with respect to chemical structural disorder." @default.
- W2956161692 created "2019-07-12" @default.
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- W2956161692 date "2019-06-25" @default.
- W2956161692 modified "2023-09-23" @default.
- W2956161692 title "Order by Chemical Disorder: Destruction of Moment Fragmentation by Charge Disorder in Nd2ScNbO7" @default.
- W2956161692 hasPublicationYear "2019" @default.
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