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- W2956296096 abstract "We demonstrate high-harmonic spectroscopy in many-electron molecules using time-dependent density-functional theory. We show that a weak attosecond-pulse-train ionization seed that is properly synchronized with the strong driving mid-infrared laser field can produce experimentally relevant high-harmonic generation (HHG) signals, from which we extract both the spectral amplitude and the target-specific phase (group delay). We also show that further processing of the HHG signal can be used to achieve molecular-frame resolution, i.e., to resolve the contributions from rescattering on different sides of an oriented molecule. In this framework, we investigate transient two-center interference in CO2 and OCS, and how subcycle polarization effects shape the oriented/aligned angle-resolved spectra." @default.
- W2956296096 created "2019-07-23" @default.
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- W2956296096 date "2019-07-01" @default.
- W2956296096 modified "2023-10-14" @default.
- W2956296096 title "High-harmonic spectroscopy of transient two-center interference calculated with time-dependent density-functional theory" @default.
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- W2956296096 doi "https://doi.org/10.1063/1.5111349" @default.
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