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- W2959685514 abstract "Deep desulfurization of fossil fuels has become urgently required because of the serious pollution by the large-scale use of fossil fuels. In this study, [PrSO3HMIm]HSO4@MIL-100(Fe) was synthesized by wet-impregnation of the ionic liquid (IL) of [PrSO3HMIm]HSO4 on MIL-100(Fe). The construction of [PrSO3HMIm]HSO4@MIL-100(Fe) was then confirmed by X-ray powder diffraction, N2 adsorption-desorption experiments, infrared spectroscopy and elemental analysis, and then applied in the oxidative desulfurization of model fuels. In comparison with the corresponding IL, [PrSO3HMIm]HSO4@MIL-100(Fe) showed an enhanced performance in the desulfurization rate of model fuels due to the increase of the mass transfer rate. Under the optimized conditions (oxidant to sulphur ratio = 25, oil to acetonitrile ratio = 1, and temperature = 60 °C), a sulphur removal rate of 99.3% was observed (initial sulphur concentration = 50 ppm). The sulphur removal of three sulphur compounds by catalytic oxidation and extraction followed the order of dibenzothiophene (DBT) > thiophene (T) > benzothiophene (BT)." @default.
- W2959685514 created "2019-07-23" @default.
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- W2959685514 date "2019-01-01" @default.
- W2959685514 modified "2023-10-01" @default.
- W2959685514 title "Deep oxidative desulfurization of model fuels catalysed by immobilized ionic liquid on MIL-100(Fe)" @default.
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- W2959685514 doi "https://doi.org/10.1039/c9ra03035b" @default.
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- W2959685514 hasPublicationYear "2019" @default.
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