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- W2959932303 abstract "The progressively improved heterobimetallic antimony transition metal complex PSbP–Pt (I1) provides superior activity in catalyzed 1,6-enyne cycloisomerization. Our DFT calculations demonstrate that the noninnocent character of the antimony ligand enhances the self-activation of the catalyst precursor through a substrate-aided intramolecular chloride migration, which triggers subsequent reaction. Designed alternative redox noninnocent active species with strong electron-withdrawing groups also show promising catalytic ability due to an electron-deficient antimony ligand, which lowers the typical reaction barrier for the cycloisomerization of 1,6-enyne." @default.
- W2959932303 created "2019-07-23" @default.
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- W2959932303 date "2019-07-08" @default.
- W2959932303 modified "2023-10-12" @default.
- W2959932303 title "Lewis Acidic PSbP Pincer Ligand in Pt-Catalyzed 1,6-Enyne Cycloisomerization: A Theoretical Study" @default.
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- W2959932303 doi "https://doi.org/10.1021/acs.joc.9b00794" @default.
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