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• W2960135159 abstract "Molecular dynamics (MD) simulations are used to measure dynamical properties of a simple bead-spring model of A-B diblock copolymer molecules, and to characterize rates and mechanisms of several dynamical processes. Dynamical properties are analyzed within the context of a kinetic population model that allows for both stepwise insertion and expulsion of individual free molecules and occasional fission and fusion of micelles. Kinetic coefficients for stepwise processes and micelle fission have been extracted from MD simulations of individual micelles. Insertion of a free surfactant molecule into a preexisting micelle is shown to be a completely diffusion-controlled process for the model studied here. Estimates are given for rates of rare events that create and destroy entire micelles by competing mechanisms involving stepwise association and dissociation or fission and fusion. Both mechanisms are shown to be relevant over the range of parameters studied here, with association and dissociation dominating in systems with more soluble surfactants and fission and fusion dominating in systems with less soluble surfactants." @default.
• W2960135159 created "2019-07-23" @default.
• W2960135159 creator A5009807848 @default.
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• W2960135159 date "2019-07-08" @default.
• W2960135159 modified "2023-09-25" @default.
• W2960135159 title "Simulation of diblock copolymer surfactants. II. Micelle kinetics" @default.
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• W2960135159 doi "https://doi.org/10.1103/physreve.100.012603" @default.
• W2960135159 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31499829" @default.
• W2960135159 hasPublicationYear "2019" @default.
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