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- W2960489944 abstract "Magnetic van der Waals materials provide an ideal platform for exploring two-dimensional magnetism of technological and scientific importance. Among them, 1T-VSe2 has been reported as one of the first room-temperature two-dimensional ferromagnets. However this conclusion remains elusive both theoretically and experimentally. By using charge self-consistent LDA+DMFT approach, suited for both itinerant and localized characters of electrons in the open-d subshells, we show that the monolayer is ferromagnetically ordered below 250K, implying the possible competition between charge density wave and ferromagnetic order. We predict that its ferromagnetism is vulnerable to interlayer coupling and extra charge dopings. The formation of local moment is attributed to the concerted effect of the quasiparticle pre-localization caused by reduced dimensionality and the electronic correlation. This study provides an important example where the reduced dimensionality is an essential factor to form local moments and subsequent magnetic orderings." @default.
- W2960489944 created "2019-07-23" @default.
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- W2960489944 date "2019-07-10" @default.
- W2960489944 modified "2023-09-24" @default.
- W2960489944 title "Sub-room temperature ferromagnetism and its nature in VSe$_2$ monolayer" @default.
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