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• W2964011165 endingPage "2118" @default.
• W2964011165 startingPage "2093" @default.
• W2964011165 abstract "We present,a new approach for predicting stable equilibrium shapes of two-dimensional crystalline islands on flat substrates, as commonly occur through solid-state dewetting of thin films. The new theory is a generalization of the widely used Winterbottom construction (i.e., an extension of the Wulff construction for particles on substrates). This approach is equally applicable to cases where the crystal surface energy is isotropic, weakly anisotropic, strongly anisotropic, and “cusped”. We demonstrate that, unlike in the classical Winterbottom approach, multiple equilibrium island shapes may be possible when the surface energy is strongly anisotropic. We analyze these shapes through perturbation analysis, by calculating the first and second variations of the total free energy functional with respect to contact locations and island shape. Based on this analysis, we find the necessary conditions for the equilibria to be stable to two-dimensional perturbations and exploit this through a generalization of the Winterbottom construction to identify all possible stable equilibrium shapes. Finally, we propose a dynamical evolution method based on surface diffusion mass transport to determine whether all of the stable equilibrium shapes are dynamically accessible. Applying this approach, we demonstrate that islands with different initial shapes may evolve into different stationary shapes and show that these dynamically determined stationary states correspond to the predicted stable equilibrium shapes, as obtained from the generalized Winterbottom construction." @default.
• W2964011165 created "2019-07-30" @default.
• W2964011165 creator A5029127277 @default.
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• W2964011165 date "2017-01-01" @default.
• W2964011165 modified "2023-10-15" @default.
• W2964011165 title "Stable Equilibria of Anisotropic Particles on Substrates: A Generalized Winterbottom Construction" @default.
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• W2964011165 doi "https://doi.org/10.1137/16m1091599" @default.
• W2964011165 hasPublicationYear "2017" @default.
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