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- W2964273326 abstract "Photoinduced biological processes occur via one photon absorption in natural light, which is weak, CW and incoherent, but are often studied in the laboratory using pulsed coherent light. Here we compare the response of a molecule to these two very different sources within a quantized radiation field picture. The latter is shown to induce coherent time evolution in the molecule, whereas the former does not. As a result, the coherent time dependence observed in the laboratory experiments will not be relevant to the natural biological process. Emphasis is placed on resolving confusions regarding this issue that are shown to arise from aspects of quantum measurement and from a lack of appreciation of the proper description of the absorbed photon." @default.
- W2964273326 created "2019-07-30" @default.
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- W2964273326 date "2011-08-31" @default.
- W2964273326 modified "2023-09-27" @default.
- W2964273326 title "Molecular Response in Coherent vs. Incoherent One Photon Absorption" @default.
- W2964273326 hasPublicationYear "2011" @default.
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