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- W2964707905 abstract "Interactions between the lattice and charge carriers can drive the formation of phases and ordering phenomena that give rise to conventional superconductivity, insulator-to-metal transitions, and charge-density waves. These couplings also play a determining role in properties that include electric and thermal conductivity. Ultrafast electron diffuse scattering (UEDS) has recently become a viable laboratory-scale tool to track energy flow into and within the lattice system across the entire Brillouin zone, and deconvolves interactions in the time domain. Here, we present a detailed quantitative framework for the interpretation of UEDS signals, ultimately extracting the phonon mode occupancies across the entire Brillouin zone. These transient populations are then used to extract momentum- and mode-dependent electron-phonon and phonon-phonon coupling constants. Results of this analysis are presented for graphite, which provides complete information on the phonon-branch occupations and a determination of the $A_1'$ phonon mode-projected electron-phonon coupling strength $langle g_{e,A_1'}^2 rangle = 0.035 pm 0.001$ eV$^2$ that is in agreement with other measurement techniques and simulations." @default.
- W2964707905 created "2019-08-13" @default.
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- W2964707905 date "2019-08-07" @default.
- W2964707905 modified "2023-09-26" @default.
- W2964707905 title "Time- and momentum-resolved phonon spectroscopy with ultrafast electron diffuse scattering" @default.
- W2964707905 hasPublicationYear "2019" @default.
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