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• W2965718598 abstract "A novel 3D bismuth-organic framework (called Bi-TBAPy) single crystal was synthesized by employing 1,3,6,8-tetrakis(p-benzoic acid)pyrene (H4TBAPy) as an organic linker. The study demonstrates that the Bi-TBAPy not only possesses good chemical stability and suitable band edge positions for promising photocatalytic H2 evolution, but it also exhibits a typical ligand-to-metal charge transfer for favorable charge separation. The photocatalytic H2 evolution rates on the as-obtained Bi-TBAPy with different cocatalysts modified were examined with triethanolamine as the sacrificial reagent. Based on this, the hydrogen evolution rate of 140 μmol h−1 g−1 was obtained on the optimized sample with a loading of 2 wt% Pt as a cocatalyst. To the best of our knowledge, this is the first bismuth-based metal-organic framework (MOF) that functions as an effective photocatalyst for photocatalytic water reduction. Our study not only adds a new member to the family of photocatalyst materials, but also reveals the importance of cocatalyst modification in improving photocatalytic activity of MOFs." @default.
• W2965718598 created "2019-08-13" @default.
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• W2965718598 date "2019-09-01" @default.
• W2965718598 modified "2023-09-25" @default.
• W2965718598 title "Development of a bismuth-based metal-organic framework for photocatalytic hydrogen production" @default.
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• W2965718598 doi "https://doi.org/10.1016/s1872-2067(19)63329-2" @default.
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