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- W2966634905 abstract "Abstract Resolving the mismatch between the practical potential window (PPW) and the available capacitive potential window of supercapacitor electrodes provides a feasible way to expand the operating voltage of supercapacitors, which further boosts energy density. Here, our research unveils a unique approach to manually control the PPW of the corresponding carbon-based supercapacitors (CSCs) by rational functionalization with amino groups. The extra pair of electrons from amino N atoms naturally adsorbs cations in the electrolyte, which rationalizes the surface charge of the carbon electrode and adjusts the PPW. A remarkable voltage expansion is achieved for CSCs, from 1.4 V to its maximum limit, 1.8 V, correspondently resulting in an approximately 1-fold increase in the energy density. Importantly, such a simple strategy endows our CSCs with an outstanding maximum energy density of 7.7 mWh cm−3, which is not only among the best values reported for thin-film CSCs but also comparable to those reported for Li thin-film batteries. These encouraging results are believed to bring fundamental insights into the nature of potential control in energy storage devices." @default.
- W2966634905 created "2019-08-13" @default.
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- W2966634905 date "2019-11-01" @default.
- W2966634905 modified "2023-10-17" @default.
- W2966634905 title "Amino functionalization optimizes potential distribution: A facile pathway towards high-energy carbon-based aqueous supercapacitors" @default.
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- W2966634905 doi "https://doi.org/10.1016/j.nanoen.2019.103987" @default.
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