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- W2966638925 abstract "In the presence of chiral phosphoramidite ligand, a palladium-catalyzed asymmetric allylic C–H alkylation of 1,4-dienes with cyclic β-keto esters has been established to afford chiral α,α-disubstituted β-keto esters in good to excellent yields, with high levels of regioselectivity, E/Z selectivity, and enantioselectivity. 1,4-Dienes bearing a wide scope of functional groups, such as ketone, chloride, ester, and amide as well, have been nicely tolerated. In addition, preliminary application of this method enables a concise formal synthesis of (−)-tanikolide." @default.
- W2966638925 created "2019-08-13" @default.
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- W2966638925 date "2019-08-06" @default.
- W2966638925 modified "2023-10-14" @default.
- W2966638925 title "Palladium-Catalyzed Asymmetric Allylic C–H Alkylation of 1,4-Dienes with Cyclic β-Keto Esters" @default.
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- W2966638925 doi "https://doi.org/10.1021/acs.organomet.9b00363" @default.
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