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• W2966706908 startingPage "104578" @default.
• W2966706908 abstract "For a supercritical solvent–solute system, as a critical end point (CEP) is approached, the solubility becomes sensitive to temperature variations. By virtue of this phenomenon, a conceptual model is proposed to combine extraction and crystal growth. CO2–naphthalene is chosen as the reference system. Theoretical optimizations suggest that the newly defined pseudo-CEPs are favorable reference states, especially those close to the lower CEP. In each near-CEP region, the performance is promoted when the CEP is approached. The temperature at the bottom wall should be higher than that at the top one to offset the stabilizing concentration gradient due to gravity and initiate double-diffusive convection in the cooperative regime. Numerical simulations confirm that the performance of the current model operating at the optimized reference state is better than the previous experimental results in terms of crystal growth rates. The conceptual model provides an efficient configuration for coupled extraction and crystal growth apparatuses." @default.
• W2966706908 created "2019-08-13" @default.
• W2966706908 creator A5041586785 @default.
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• W2966706908 date "2019-11-01" @default.
• W2966706908 modified "2023-09-26" @default.
• W2966706908 title "Coupled extraction and crystal growth in supercritical solutions: Model and theory" @default.
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• W2966706908 doi "https://doi.org/10.1016/j.supflu.2019.104578" @default.
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