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• W2967012258 abstract "In glass-forming liquids there is a secondary β-relaxation that bears a strong connection to structural α-relaxation and is of fundamental importance. It is natural to inquire whether ionic conductivity relaxation in ionic conductors possesses the same property. This question has not been answered before because β-relaxation had not been found or resolved in all kinds of ionic conductors. Herein, we investigate ion dynamics in supercooled and glassy states of four 1-butyl-1-methylpyrrolidinium based ionic liquids differing significantly in the size and strength of interactions between ionic species. Despite these differences, all four samples exhibit a prominent β-relaxation with dynamics strongly connected to the primary conductivity relaxation. The general results indicate that β-relaxation is indispensable as a precursor in generating the cooperative conductivity relaxation and in turn the dc conductivity. The novel findings have an impact on the research of conductivity relaxation in the broad field of ionic conductors." @default.
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• W2967012258 date "2019-08-16" @default.
• W2967012258 modified "2023-09-27" @default.
• W2967012258 title "Evidence of a Fundamental Mechanism Governing Conductivity Relaxation in Room-Temperature Ionic Liquid" @default.
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• W2967012258 doi "https://doi.org/10.1021/acs.jpcc.9b07578" @default.
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