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• W2967381562 abstract "Abstract The nature of the electronic interface between a nanotube and solvated ions in a liquid electrolyte is governed by two distinct physical phenomena: quantum and chemical. The quantum component arises from the sharply varying electronic density of states and the chemical component arises from ion screening and diffusion. Here, using an integrated on-chip shield technology, we measure the capacitance of one to a few nanotubes quantitatively as a function of both bias potential (from −0.7 V to 0.3 V) and ionic concentration (from 10 mM to 1 M KCl) at room temperature. We determine the relative contributions of the quantum and electrochemical capacitance, and confirm the measurements with theoretical models. This represents an important measurement of the quantum effects on capacitance in reduced dimensional systems in contact with liquid electrolytes, an important and emerging theme in the interface between nanotechnology, energy, and life." @default.
• W2967381562 created "2019-08-22" @default.
• W2967381562 creator A5016807370 @default.
• W2967381562 creator A5068885142 @default.
• W2967381562 date "2019-08-09" @default.
• W2967381562 modified "2023-10-14" @default.
• W2967381562 title "Measurement of the combined quantum and electrochemical capacitance of a carbon nanotube" @default.
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• W2967381562 doi "https://doi.org/10.1038/s41467-019-11589-9" @default.
• W2967381562 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6689019" @default.
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• W2967381562 hasPublicationYear "2019" @default.
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