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• W2967478304 abstract "Abstract Dye molecules pre‐anchored on titanium oxo clusters (dye‐TOCs) are attractive as model compounds of dye‐sensitized titanium oxide. To investigate the effects of the dye ligand structures of the dye‐TOCs on photocurrent conversion, a series of dye‐TOCs with the same Ti 6 core structure and different antenna ligands (L) was synthesized and characterized crystallographically. The TOCs have the same structural formula of [Ti 6 O 4 L 2 (O 3 PPh) 2 (O i Pr) 10 ]. Two types of dyes with para ‐ or meta ‐substituted structures were designed and used as the ligands. The results show that charge transfer from the donor group to the TiO core of the TOCs with the para ‐substituted ligands is stronger than those with the meta ‐substituted ligands. The steric effect of the ligands also greatly influences the photocurrent density. Larger branched structures of the dye ligands reduce the coverage density of the dye‐TOCs on TiO 2 electrodes and also weaken the effective covalent bonding of the dye‐TOCs on the electrode, and consequently, the photocurrent is decreased." @default.
• W2967478304 created "2019-08-22" @default.
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• W2967478304 date "2019-08-27" @default.
• W2967478304 modified "2023-09-25" @default.
• W2967478304 title "A Series of Ti ₆ Oxo Clusters Anchored with Arylamine Dyes: Effect of Dye Structures on Photocurrent Responses" @default.
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• W2967478304 doi "https://doi.org/10.1002/asia.201900921" @default.
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