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- W2967721879 abstract "In a Kitaev spin liquid, electron spins can break into fractional particles known as Majorana fermions and Z$_2$ fluxes. Recent experiments have indicated the existence of such fractional particles in a two-dimensional Kitaev material candidate, $alpha$-RuCl$_3$. These exotic particles can be used in topological quantum computations when braided within their lifetimes. However, the lifetimes of these particles, critical for applications in topological quantum computing, have not been reported. Here we study ultrafast dynamics of photoinduced excitations in single crystals of $alpha$-RuCl$_3$ using pump-probe transient grating spectroscopy. We observe intriguing photoexcited nonequilibrium states in the Kitaev paramagnetic regime between $T_N$~7 K and $T_H$~100 K, where $T_N$ is the N'eel temperature and $T_H$ is set by the Kitaev interaction. Two distinct lifetimes are detected: a longer lifetime of ~50 ps, independent of temperature; a shorter lifetime of 1-20 ps, with a strong temperature dependence, $T^{-1.40}$. We analyze the transient grating signals using coupled differential equations and propose that the long and short lifetimes are associated with fractional particles in the Kitaev paramagnetic regime, Z$_2$ fluxes and Majorana fermions, respectively." @default.
- W2967721879 created "2019-08-22" @default.
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- W2967721879 date "2019-08-13" @default.
- W2967721879 modified "2023-09-26" @default.
- W2967721879 title "Ultrafast dynamics of fractional particles in $alpha$-RuCl$_3$" @default.
- W2967721879 hasPublicationYear "2019" @default.
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