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- W2968009008 abstract "The loading amount of Ba promoter in the 15 wt% Co/CeO2 catalyst system was varied from 0 wt% to 3 wt%, and the resulting catalysts were used for the high-temperature water-gas shift (HTS) reaction. The catalysts were prepared by the incipient wetness co-impregnation method and studied through various characterization techniques such as X-ray diffraction, Brunauer–Emmet–Teller measurements, CO–chemisorption, H2–temperature programmed reduction, X-ray photoelectron spectroscopy, and transmission electron microscopy. The doping of Ba as a promoter in the optimal amount (1–2 wt%) improves the reducibility of the catalyst and enhances its sintering resistance. However, the doping of an excessive amount (≥3 wt%) of the promoter lowers the reducibility of the catalyst, resulting in the instability of the active phase (Co0). Overall, the 1% BaCo/CeO2 catalyst exhibited the best performance even at a severe reaction condition (CO conc. = 38%, GHSV = 143,000 h−1) owing to the strong resistance to the sintering and high stability of the active phase." @default.
- W2968009008 created "2019-08-22" @default.
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- W2968009008 date "2020-01-01" @default.
- W2968009008 modified "2023-09-25" @default.
- W2968009008 title "Increase in stability of BaCo/CeO2 catalyst by optimizing the loading amount of Ba promoter for high-temperature water-gas shift reaction using waste-derived synthesis gas" @default.
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- W2968009008 doi "https://doi.org/10.1016/j.renene.2019.08.050" @default.
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