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- W2968273802 abstract "We investigated the self-assembled structures and photoresponsive and crystallization behaviors of supramolecules composed of 4-methoxy-4′-hydroxyazobenzene (Azo) molecules and polyethylene glycol (PEG) that were formed through hydrogen-bonding interactions. The Azo/PEG complexes exhibited the characteristics of photoresponse and crystallization, which originated from Azo and PEG, respectively. When Azo/PEG complexes were dissolved in solvents, hydrogen-bonding interaction hindered the rotation and inversion of mesogens, causing a reduction in the photoisomerization rate compared with the photoisomerization rate of the neat Azo. The confinement of Azo/PEG complexes in thin films further resulted in a substantial decrease in the photoisomerization rate but an increase in the amounts of H-aggregated and J-aggregated mesogens. Regarding PEG crystallization, ultraviolet irradiation of Azo/PEG complexes increased the quantity of high-polarity cis isomers, which improved the compatibility between mesogens and PEG, subsequently increasing the crystallization temperature of PEG. Moreover, the complexation of Azo and PEG induced microphase separation, forming a lamellar morphology. Within the Azo-rich microphases, mesogens aggregated to form tilted monosmectic layers. By contrast, PEG crystallization within the PEG-rich microphases was hard confined, indicating that the domain size of the lamellar morphology was unchanged during PEG crystallization." @default.
- W2968273802 created "2019-08-22" @default.
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- W2968273802 date "2019-08-16" @default.
- W2968273802 modified "2023-10-14" @default.
- W2968273802 title "Hydrogen Bonding-Induced Assembled Structures and Photoresponsive Behavior of Azobenzene Molecule/Polyethylene Glycol Complexes" @default.
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- W2968273802 doi "https://doi.org/10.3390/polym11081360" @default.
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