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• W2968282013 abstract "Abstract An improved kinetic model for the radical polymerization of N ‐vinyl‐pyrrolidone (NVP) in aqueous medium is developed. Quantum chemical simulations reveal that the transfer to polymer is of minor importance whereas the transfer to monomer by hydrogen abstraction in 3‐position of the pyrrolidone ring leads to a radical with a double bond which initiates a new chain bearing a terminal double bond (TDB). The resulting dead chains with one, two, or more TDB are the main source for a strong increase of molar mass in batch reactors at high conversion due to long chain branching and crosslinking. This can be a source for gel formation and fouling in continuous reactors." @default.
• W2968282013 created "2019-08-22" @default.
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• W2968282013 date "2019-08-13" @default.
• W2968282013 modified "2023-10-18" @default.
• W2968282013 title "Side Reactions in Aqueous Phase Polymerization of <i>N</i> ‐Vinyl‐Pyrrolidone as Possible Source for Fouling" @default.
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• W2968282013 doi "https://doi.org/10.1002/mren.201900021" @default.
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