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• W2968373334 abstract "The end-oxygens (end-O) of metal–oxygen chains on transition-metal (TM) surfaces play a vital role in the decomposition of H-contained molecules, such as H2O and alcohols. However, the achievement of high density of ordered end-O structures on TM surfaces is still challenging so far. In this paper, based on the evidence of ultrahigh vacuum-Fourier transform infrared spectroscopy and density functional theory calculations, we successfully prepared the high density of ordered end-O structures on Ni(110) surfaces through breaking the long Ni–O chains to short Ni–O chains by NO adsorption on (2 × 1)Ni–O/Ni(110) reconstructed surfaces. The mechanism of end-O formation has been interpreted: at low NO coverage at 90 K, NO molecules tiltedly adsorb on Ni atoms in Ni–O chains causing a strong distortion; when NO coverage is increased close to saturation (∼0.5 ML), the accumulated stress of Ni–O chains finally breaks the Ni–O bonds, resulting in the release of the host Ni atoms in Ni–O chains to the hollow sites and the formation of two end-O for each released Ni. Furthermore, the ordering of end-O structures on Ni(110) surfaces can be greatly enhanced by the annealing of the sample to 250 K. Such an approach to prepare the high density of ordered end-O structures is expectedly applied to other TM surfaces." @default.
• W2968373334 created "2019-08-22" @default.
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• W2968373334 date "2019-08-14" @default.
• W2968373334 modified "2023-10-14" @default.
• W2968373334 title "High Density of End-Oxygens Induced by NO Adsorption on (2 × 1)Ni–O/Ni(110) Surfaces" @default.
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• W2968373334 doi "https://doi.org/10.1021/acs.jpcc.9b05658" @default.
• W2968373334 hasPublicationYear "2019" @default.
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