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- W2968486992 abstract "Synthesis of cyclic carbonates via CO2 cycloaddition reaction with epoxides is one of the promising strategies to valorize greenhouse gas CO2, thereby fixing it to the value-added chemicals. In this study, uniform copper oxide nanoparticles (Cu2O, Cu4O3) with variable oxidation states are stabilized by functionalized covalent organic frameworks (COF) and effectively utilized as a catalyst for the synthesis of cyclic carbonates under ambient temperature and atmospheric pressure. Characterization techniques e.g. powdered X-ray Diffraction (PXRD), high resolution transmission electron microscopy (HRTEM), Fourier transform infrared (FT-IR) and nitrogen physisorption (BET) coupled with DFT studies predict that the copper oxide nanoparticles are anchored on the mesochannels of covalent organic frameworks through a covalent-coordinate linkage. The catalyst exhibits significantly high turn over numbers (TON, order of 105) and more than 99% selectivity towards synthesis of cyclic carbonates with exceptional recyclability." @default.
- W2968486992 created "2019-08-22" @default.
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- W2968486992 date "2019-12-01" @default.
- W2968486992 modified "2023-09-28" @default.
- W2968486992 title "CuxOy@COF: An efficient heterogeneous catalyst system for CO2 cycloadditions under ambient conditions" @default.
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- W2968486992 doi "https://doi.org/10.1016/j.jcou.2019.07.036" @default.
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