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- W2969175048 abstract "Abstract Suzuki coupling is of paramount importance in C−C coupling reactions. However, Suzuki coupling reactions are generally catalyzed by homogeneous catalysts under thermal heating, which results in difficulties in the catalyst separation and consumes a relatively large amount of energy. g ‐C 3 N 4 /Pd has been successfully prepared for photocatalytic Suzuki coupling reactions. The g ‐C 3 N 4 /Pd is prepared through the reduction of a Pd source in the presence of g ‐C 3 N 4 . The Pd is found to exist as Pd nanoparticles and Pd(II) species on g ‐C 3 N 4 . Owing to the good light absorption of g ‐C 3 N 4 and the excellent catalytic activity of the Pd species, the g ‐C 3 N 4 /Pd shows an excellent photocatalytic performance in Suzuki coupling reactions with a TOF of 47.3 h −1 , which is almost twice that of a commercial homogeneous catalyst Pd(PPh 3 ) 4 , under thermal heating. Moreover, g ‐C 3 N 4 /Pd displays very good recyclability and wide applicability for Suzuki coupling reactions. Our findings provide a green and sustainable method for the catalysis of Suzuki coupling reactions." @default.
- W2969175048 created "2019-08-22" @default.
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- W2969175048 date "2019-08-01" @default.
- W2969175048 modified "2023-10-17" @default.
- W2969175048 title "Graphitic Carbon Nitride (g‐C<sub>3</sub>N<sub>4</sub>) Supported Palladium Species: An Efficient Heterogeneous Photocatalyst Surpassing Homogeneous Thermal Heating Systems for Suzuki Coupling" @default.
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- W2969175048 doi "https://doi.org/10.1002/cplu.201900360" @default.
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