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• W2969226800 abstract "We determine experimentally the excited-state interatomic forces in photoexcited bismuth. The forces are obtained by a constrained least-squares fit of the excited-state dispersion obtained by femtosecond time-resolved x-ray diffuse scattering to a fifteen-nearest neighbor Born-von Karman model. We find that the observed softening of the zone-center $A_{1g}$ optical mode and transverse acoustic modes with photoexcitation are primarily due to a weakening of three nearest neighbor forces along the bonding direction. This provides a more complete picture of what drives the partial reversal of the Peierls distortion previously observed in photoexcited bismuth." @default.
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• W2969226800 date "2021-05-18" @default.
• W2969226800 modified "2023-10-14" @default.
• W2969226800 title "Measurements of nonequilibrium interatomic forces using time-domain x-ray scattering" @default.
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• W2969226800 doi "https://doi.org/10.1103/physrevb.103.l180101" @default.
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