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- W2969267560 endingPage "100132" @default.
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- W2969267560 abstract "The development of bifunctional cathode catalysts with advantages such as high activity, low cost, and high durability is highly desirable and challenging for zinc-air batteries (ZABs) in energy applications. In this work, a novel type of bifunctional catalyst (CoPx/Co-Nx[email protected]) simultaneously effective for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) was prepared via a simplified all-in-one phosphorization-carbonization synthesis, which is distinctively different from the previously reported carbonization and postphosphorization route. With the integration of efficient catalytic factors such as Co-Nx-C–coordinated moieties, cobalt phosphide, graphitic carbon shells, as well as a supportive and conductive matrix, the as-prepared CoPx/Co-Nx[email protected] exhibits high catalytic activity for ORR and OER in 0.1 M KOH, with an output positive onset potential of 0.92 V vs reversible hydrogen electrode (RHE) for ORR and a low potential of 1.69 V vs RHE at 10 mA cm−2 for OER. Remarkably, the assembled liquid and all-solid-state ZAB based on the as-prepared CoPx/Co-Nx[email protected] showed superior cycling performance than the results of its Pt/C-based counterparts and some recently reported cobalt phosphide–based ZABs. The good flexibility and reversibility of the all-solid-state ZAB also verified its feasibility in applications such as wearable electronics." @default.
- W2969267560 created "2019-08-29" @default.
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- W2969267560 date "2019-06-01" @default.
- W2969267560 modified "2023-10-12" @default.
- W2969267560 title "Microwave-assisted synthesis of carbon nanotubes threaded core-shell CoP /Co-N -C@CNT and its performance as an efficient bifunctional oxygen catalyst for the rechargeable zinc-air battery" @default.
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- W2969267560 doi "https://doi.org/10.1016/j.mtphys.2019.100132" @default.
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