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- W2969657629 endingPage "118115" @default.
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- W2969657629 abstract "Surface functionalization is closely associated with the light harvesting and the charge separation, transfer, and injection efficiencies of water-splitting photoelectrode. Here, a dual-phase photoetching template with hierarchical structure, polyphenylsilsequioxane nanopillars and bicontinuous polyphenylsilsequioxane + polystyrene network layer, is patterned on the Si photoanode via a spinodal phase separation mechanism. Controllably photoetching the polymer template allows us to physically deposit functional layers with tunable nanostructures from net to dispersed dot. As a demonstration, the broken Ni/NiOx net modified Si photoanode exhibits a low onset potential of 0.93 VRHE, a high saturated photocurrent density of 40 mA cm−2 and a stability of 50 h in 1.0 M K-borate under AM1.5 G illumination, resulting from the inhomogeneous barrier height driven efficient charge extraction and low light loss by the dispersed surface modification. The proposed dual-phase lithographic template may open a new avenue to easily assemble functional layers on photoelectrodes for efficient solar energy conversion." @default.
- W2969657629 created "2019-08-29" @default.
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- W2969657629 date "2019-12-01" @default.
- W2969657629 modified "2023-10-14" @default.
- W2969657629 title "A hierarchical dual-phase photoetching template route to assembling functional layers on Si photoanode with tunable nanostructures for efficient water splitting" @default.
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- W2969657629 doi "https://doi.org/10.1016/j.apcatb.2019.118115" @default.
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