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- W2969722020 abstract "In this article, we present our studies on the mass-transfer of Br species existing in an acidic aqueous solution containing quaternary ammonium bromide (QBr) during electro-oxidation of Br−. We found that the mass-transfer of quaternary ammonium polybromide (QBr2n+1) droplets toward a Pt ultramicroelectrode (UME) are mainly governed by diffusion, although their migration is not negligible. We further revealed that the migration of Br− in a QBr2n+1 droplet significantly affects the current associated with the electro-oxidation of Br− during the collision of the droplet on a Pt UME. Finally, we observed current spikes in which the current decayed and reached a certain steady state with a non-zero value. These were interpreted based on Br−-transfer at the interface between water and a QBr2n+1 droplet (water|QBr2n+1) using finite element analysis. The presented electrochemical analyses would be potentially important to understand the operating mechanism of redox flow batteries (RFBs) using Br−/Br2 as a half redox reaction to inhibit the self-discharge that occurs during the charging process." @default.
- W2969722020 created "2019-08-29" @default.
- W2969722020 creator A5079206867 @default.
- W2969722020 creator A5085583792 @default.
- W2969722020 date "2019-12-01" @default.
- W2969722020 modified "2023-10-16" @default.
- W2969722020 title "Understanding the mass-transfer of Br species in an aqueous and quaternary ammonium polybromide biphasic system via particle-impact electrochemical analysis" @default.
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- W2969722020 doi "https://doi.org/10.1016/j.jiec.2019.08.028" @default.
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