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- W2970029852 abstract "• Carbon neutral methane production by chemical conversion of CO 2 waste flue gases. • Using renewable energy in a circular economy scheme. • Plasmas generation by electrical discharges on CO 2 +H 2 gas mixtures. • New emerging catalysts development in chemical engineering. • Plasma-assisted CO 2 conversion on CH 4 fuel. An experimental study aiming at reusing CO 2 and implementing a validated laboratory technology based on a prototype methanation reactor (ProGeo) producing carbon neutral methane through the chemical conversion of CO 2 waste flue gases using renewable energy in a circular economy scheme, is presented. ProGeo is able to produce a CH 4 flux of 1 Nm 3 /h, using the Sabatier reaction at high pressure (1.5–3 bar) and temperature (200–400 °C) with a solid phase catalyst. Furthermore, the investigation of a new methanation pathway by exploring mechanisms involving a plasma generation by electrical discharges on CO 2 +H 2 gas mixtures has been undertaken. Obtained results indicate the formation of hydrocarbons as methane, formic acid and/or dimethyl ether as well as small amounts of HCO + , H 2 CO + , H 3 CO + , HCO 2 + ions. These ionic species together with CO + and O + ions, having a very high kinetic energy content, should increase the chemical reactivity of generated plasmas playing a pivotal role in the plasma-assisted CO 2 conversion on CH 4 fuel. Further experimental work is in progress to optimize the experimental conditions of the CO 2 methanation process via alternative microscopic mechanisms, using plasma assisted catalyzed reactions that are of great importance in new emerging catalysts development in chemical engineering." @default.
- W2970029852 created "2019-09-05" @default.
- W2970029852 creator A5017358294 @default.
- W2970029852 date "2020-05-01" @default.
- W2970029852 modified "2023-09-24" @default.
- W2970029852 title "Fuel production from waste CO2 using renewable energies" @default.
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- W2970029852 doi "https://doi.org/10.1016/j.cattod.2019.08.041" @default.
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