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- W2970096127 abstract "Abstract HKUST-1 nanocrystals with large accessible surface areas and high porosity were functionalized with amine groups and incorporated into polymer matrices to form mixed-matrix membranes for application in CO2 capture. This gas permeation study reveals that pristine HKUST-1 nanocrystals are able to increase the gas permeabilities of polymer membranes with no noticeable effect on CO2/N2 selectivity as a result of their high porosity and large pore dimensions. Contrarily, 20 wt% amine-functionalized HKUST-1 can improve the CO2/N2 selectivity of polymer membranes by as much as 38%. As shown in a detailed analysis of the diffusivity-solubility, the amine-functionalized HKUST-1 suppressed N2 solubility and diffusivity but enhanced CO2 diffusivity. This resulted in an increased CO2/N2 perm-selectivity. Meanwhile, the pristine HKUST-1 nanocrystals increased the diffusivity and solubility of both species in a non-selective manner. These results indicate the feasibility of tuning the CO2 separation performance of mixed-matrix membranes by introducing amine functionality into the filler." @default.
- W2970096127 created "2019-09-05" @default.
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- W2970096127 date "2019-12-01" @default.
- W2970096127 modified "2023-10-18" @default.
- W2970096127 title "Enhancing the CO2 separation performance of polymer membranes via the incorporation of amine-functionalized HKUST-1 nanocrystals" @default.
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- W2970096127 doi "https://doi.org/10.1016/j.micromeso.2019.109680" @default.
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