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- W2973008384 abstract "The direct synthesis of hydrogen peroxide using sustainable energy and molecular oxygen is a promising alternative approach to the conventional batch synthesis. Here we present a manganese and nitrogen co-doped carbon material which catalyzes the selective reduction of dioxygen in an acidic environment to hydrogen peroxide. The onset potential is close to 0.7 V, with >98% H2O2 selectivity in the range of 0.7–0.5 V vs RHE. This is the highest reported to date, outperforming many bimetallic noble metal catalysts. Besides, this doped carbon material is hierarchically porous, featuring both a large mesopore volume (4.54 mL g−1) and a high specific surface area (1333 m2 g−1). This enables the effective adsorption of bulky organics such as methylene blue (385 mg g−1). Combined with the formation of hydroxyl radicals during electrochemical H2O2 generation, this material also enables the efficient electrochemical degradation of methylene blue, as evidenced by in situ UV–vis spectrometry." @default.
- W2973008384 created "2019-09-19" @default.
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- W2973008384 date "2019-12-01" @default.
- W2973008384 modified "2023-10-17" @default.
- W2973008384 title "Efficient oxygen reduction to H2O2 in highly porous manganese and nitrogen co-doped carbon nanorods enabling electro-degradation of bulk organics" @default.
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- W2973008384 doi "https://doi.org/10.1016/j.carbon.2019.09.034" @default.
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