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- W2973694097 abstract "Abstract An efficient route to chemically functionalize reduced graphene oxide (rGO) with ruthenium organometallic compounds and the subsequent anchorage of Pt nanoparticles is reported. Two organometallic complexes, [(η 6 ‐C 6 H 5 OCH 2 CH 2 OH) RuCl 2 ] 2 ( Ru‐dim ) and [(η 6 ‐C 6 H 4 (CHMe 2 )Me)RuCl 2 ] 2 ( Ru‐cym ), as well as commercial RuCl 3 ⋅ XH 2 O ( Ru‐com ) have been synthetized an used as functionalizing agents. By implementing a conventional polyol synthesis method, the Pt/rGO Ru‐dim , Pt/rGO Ru‐cym , Pt/rGO Ru‐com and Pt/rGO nanocatalysts have been synthetized. Characterization by XRD indicates that the presence of Ru leads to the formation of Pt−Ru alloyed phases due to overlapping of Pt fcc and Ru hcp reflections. When characterized for the methanol oxidation reaction (MOR) in acid media, Pt/rGO Ru‐dim reached a mass current density of 491.49 mA mg Pt −1 , higher than those generated by the other nanocatalysts. The results show that the functionalization of rGO with Ru‐dim remarkably increases the catalytic activity of Pt for the MOR, suggesting Pt−Ru metal−metal interactions that promotes the anodic reaction." @default.
- W2973694097 created "2019-09-26" @default.
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- W2973694097 date "2019-09-16" @default.
- W2973694097 modified "2023-10-18" @default.
- W2973694097 title "Functionalizing Reduced Graphene Oxide with Ru‐Organometallic Compounds as an Effective Strategy to Produce High‐Performance Pt Nanocatalysts for the Methanol Oxidation Reaction" @default.
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- W2973694097 doi "https://doi.org/10.1002/celc.201901190" @default.
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