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• W2975437006 abstract "A single-crystal-to-single-crystal (SCSC) photodimerization is achieved using Au(I) coordination and aurophilic interactions. The rigid Au2(dppbz)(CF3COO)2 precursor (dppbz = 1,2-bis(diphenylphosphino)benzene) self-assembles with 1,2-trans-bis(4-pyridyl)ethylene (bpe) to afford a discrete [Au4(dppbz)2(bpe)2]4+ macrocycle in the solid state. The alkene undergoes a [2 + 2] photocycloaddition reaction. The photoreaction proceeds via a rare SCSC transformation in quantitative yield that generates [Au4(dppbz)2(4,4'-tpcb)]4+ (4,4'-tpcb = rctt-tetrakis(4-pyridyl)cyclobutane) stereoselectively. Mechanical strain induced by the photoreaction is evidenced by the formation of ramp features on single-crystal surfaces using scanning electron microscopy." @default.
• W2975437006 created "2019-10-03" @default.
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• W2975437006 date "2019-09-25" @default.
• W2975437006 modified "2023-09-24" @default.
• W2975437006 title "Exploiting Aurophilic Interactions in a [2 + 2] Photocycloaddition: Single-Crystal Reactivity with Changes to Surface Morphology" @default.
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• W2975437006 doi "https://doi.org/10.1021/acs.inorgchem.9b01306" @default.
• W2975437006 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31553589" @default.
• W2975437006 hasPublicationYear "2019" @default.
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