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- W2976310900 abstract "Abstract A novel template‐free Cp*Rh‐based molecular Solomon link has been established through selection of the flexible ligand L as a linker and the half‐sandwich rhodium(III) dinuclear fragment B1 as a rigid capping unit. Furthermore, we demonstrate that the self‐assembly of the Solomon link based on the flexible ligand is both solvent‐ and concentration‐dependent: the Solomon link is formed in concentrated methanolic solutions, whereas formation of a dinuclear trapezoidal rectangle is favored at low concentrations or in acetonitrile or DMF solutions. Remarkably, alteration of the solvent or concentration can promote a unique and dynamic interconversion between the two molecular species, accompanying conformational change of the ligand. The synthetic outcomes are supported by single‐crystal X‐ray diffraction analysis." @default.
- W2976310900 created "2019-10-03" @default.
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- W2976310900 date "2019-11-06" @default.
- W2976310900 modified "2023-09-27" @default.
- W2976310900 title "Dynamic Interconversion between Solomon Link and Trapezoidal Metallacycle Ensembles Accompanying Conformational Change of the Linker" @default.
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- W2976310900 doi "https://doi.org/10.1002/chem.201904196" @default.
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