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• W2976353590 abstract "A series of new ternary antimonides Ln2Pd9Sb3 (Ln = La, Pr, Nd, Sm) was synthesized from pure constituents. The crystal structure of all compounds was determined by X-ray powder diffraction. These compounds are isotypic with the Сe2Pd9Sb3 structure (anti-type to the ternary gallide Y2Co3Ga9, space group Cmcm): а = 13.7772 (6), b = 8.0642 (3), c = 9.3967 (4) Å for La2Pd9Sb3; а = 13.7392 (6), b = 8.0146 (3), c = 9.3215 (4) Å for Pr2Pd9Sb3; а = 13.7208 (5), b = 7.9983 (3), c = 9.3016 (3) Å for Nd2Pd9Sb3; а = 13.6957 (7), b = 7.9686 (4), c = 9.2700 (5) Å for Sm2Pd9Sb3. The electronic structures of Ln2Pd9Sb3 were analyzed using the tight-binding extended Hückel method on cerium representative. The analysis of the magnetic properties shows that the Ln2Pd9Sb3 (Ln = La, Nd, Pr, and Sm) compounds are paramagnetic down to a very low temperature. Curie-Weiss paramagnetic temperature are small and range from between −6 and −1 K. The Sm and Pr containing phases exhibits the largest ordering temperature of 6.8 and 6.2 K, respectively. The Ce containing phase also orders magnetically below 4 K in contrast to the La one (which remains paramagnetic even at 2 K), thus indicating that Ce is carrying an ordered magnetic moment. At 2 K, the magnetization curves of these compounds do not saturate easily even in applied fields up of 10 T." @default.
• W2976353590 created "2019-10-03" @default.
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• W2976353590 date "2020-01-01" @default.
• W2976353590 modified "2023-10-13" @default.
• W2976353590 title "Ternary antimonides Ln2Pd9Sb3 (Ln = La, Ce, Nd, Pr, and Sm): Crystal, electronic structure, and magnetic properties" @default.
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• W2976353590 doi "https://doi.org/10.1016/j.jallcom.2019.152428" @default.
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