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- W2977740077 abstract "We show that off resonance time-resolved Kerr rotation (TRKR) is a quantitatively accurate tool to measure spin dynamics by demonstrating that TRKR scans yield essentially identical temporal profiles when the probe energy is tuned far below, far above, and on resonance with the bandgap. We further show that the observed symmetry of the Kerr rotation with respect to probe energy detuning is inconsistent with time-dependent perturbation theory in the simplest case and resolve the discrepancy by recognizing that the optical lifetime decreases with excess energy above the band edge transition.We show that off resonance time-resolved Kerr rotation (TRKR) is a quantitatively accurate tool to measure spin dynamics by demonstrating that TRKR scans yield essentially identical temporal profiles when the probe energy is tuned far below, far above, and on resonance with the bandgap. We further show that the observed symmetry of the Kerr rotation with respect to probe energy detuning is inconsistent with time-dependent perturbation theory in the simplest case and resolve the discrepancy by recognizing that the optical lifetime decreases with excess energy above the band edge transition." @default.
- W2977740077 created "2019-10-10" @default.
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- W2977740077 date "2019-09-30" @default.
- W2977740077 modified "2023-09-24" @default.
- W2977740077 title "Accuracy and form of off-resonance time-resolved Kerr rotation spectroscopy" @default.
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- W2977740077 doi "https://doi.org/10.1063/1.5117142" @default.
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