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• W2978637092 abstract "Abstract Poly(3,4-ethylenedioxythiophene) (PEDOT) and single-walled carbon nanotubes (SWCNTs) are promising thermoelectric materials that exhibit flexibility and high performance. To realize improved structural and thermoelectric properties, we fabricated PEDOT/SWCNT bilayers consisting of drop-cast SWCNTs and electropolymerized PEDOT. We prepared two types of PEDOT layers using electrolyte solvents of water/methanol (Sample A) and acetonitrile (Sample B). Sample B achieved a flexible freestanding state, whereas Sample A was broken with part of the sample remaining on the substrate. Scanning electron microscopy revealed that the PEDOT layer in Sample A filled the gaps between the SWCNT bundles. The PEDOT layer in Sample B consisted of chain-like structures that mostly covered the surface of the SWCNT layer, which were speculated to increase the strength of the freestanding state. The structural properties of the bilayers were examined using Fourier transform infrared spectroscopy, Raman spectroscopy, and X-ray photoelectron spectroscopy. Although slight structural differences were observed between Samples A and B, both samples exhibited the characteristics of PEDOT and SWCNTs. Measurement of the thermoelectric properties near 300 K afforded power factors of 12.5 and 13.9 μW/(m·K2) for Samples A and B, respectively. Therefore, we demonstrated the successful fabrication of freestanding PEDOT/SWCNT bilayers (Sample B) with relatively high thermoelectric performance." @default.
• W2978637092 created "2019-10-10" @default.
• W2978637092 creator A5012698520 @default.
• W2978637092 creator A5043751841 @default.
• W2978637092 date "2020-01-01" @default.
• W2978637092 modified "2023-09-29" @default.
• W2978637092 title "Freestanding bilayers of drop-cast single-walled carbon nanotubes and electropolymerized poly(3,4-ethylenedioxythiophene) for thermoelectric energy harvesting" @default.
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• W2978637092 doi "https://doi.org/10.1016/j.orgel.2019.105478" @default.
• W2978637092 hasPublicationYear "2020" @default.
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