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- W2978644240 abstract "Although lithium-sulfur batteries are promising environmentally friendly and low-cost energy storage devices with high energy densities, many obstacles such as poor conductivity, volume expansion and the shuttle effect still limit their large-scale commercialization. In this work, a 2D sandwich-like α-ZrP/polypyrrole (α-ZrP/PPy) material with a nanosheet structure was designed as a sulfur host. The material can provide unique ion transfer channels for the rapid transfer of Li+ ions and catalytically promote the conversion of lithium polysulfides (LiPSs). Moreover, the α-ZrP nanosheets provides a true covalent anchor for sulfur species, whereas the PPy builds a physical barrier and forms a conductive network for accelerating the electron transport and promoting the electrochemical performance. In addition, the moderate catalytic activity and true sulfur confinement effect of α-ZrP were confirmed by experiments and theoretical calculations. The α-ZrP/PPy@S cathode exhibits a highly reversible capacity of 727.2 mAh g-1 even at a high current density of 5 C, offering a novel cathode material for high performance Li-S batteries." @default.
- W2978644240 created "2019-10-10" @default.
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- W2978644240 date "2019-11-07" @default.
- W2978644240 modified "2023-10-16" @default.
- W2978644240 title "2D Sandwich‐Like α‐Zirconium Phosphate/Polypyrrole: Moderate Catalytic Activity and True Sulfur Confinement for High‐Performance Lithium–Sulfur Batteries" @default.
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- W2978644240 doi "https://doi.org/10.1002/cssc.201902227" @default.
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