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• W2978930221 abstract "Chemical protection is an essential tool in synthetic chemistry, which involves blocking reactive sites on a molecule through covalent bonds. Physical approaches, such as encapsulation and host-mediated protection, have emerged as interesting alternatives that use steric bulk to inhibit reactivity. Here, we report the protection of a redox-active viologen through its incorporation into mechanically interlocked molecules (MIMs), namely hetero[4]rotaxanes. The viologen was confined inside a host cavity and flanked by two mechanical stoppers, which allowed for permanent and transient protection. Deprotection occurred on-demand via an unstoppering process, triggered by a proton transfer, polarity effect, or a thermal stimulus. We anticipate that permanent and transient mechanical stoppering could be incorporated into devices to function as molecular probes, transport/delivery systems, or stimuli-controlled degradable materials." @default.
• W2978930221 created "2019-10-10" @default.
• W2978930221 creator A5008803440 @default.
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• W2978930221 date "2019-01-01" @default.
• W2978930221 modified "2023-10-18" @default.
• W2978930221 title "Programming permanent and transient molecular protection <i>via</i> mechanical stoppering" @default.
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• W2978930221 doi "https://doi.org/10.1039/c9sc03744f" @default.
• W2978930221 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6988755" @default.
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• W2978930221 hasPublicationYear "2019" @default.
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