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- W2979299505 abstract "Abstract We report in this article a cascade reaction strategy for the synthesis of complex N‐heterocyclic compounds with contiguous and tetrasubstituted stereogenic carbons. Under the sequential catalysis of a chiral binol–Ti complex and BF 3 , cyclopentanone‐derived tertiary enamides undergo an enantioselective enamine addition to ketone carbonyls followed by diastereoselective trapping of the resulting acyliminiums by electron‐rich aryl moieties to furnish four‐ and five‐membered ring‐fused N‐heterocyclic products as the sole diastereomers in high yields with up to 99 % ee ." @default.
- W2979299505 created "2019-10-18" @default.
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- W2979299505 date "2019-12-05" @default.
- W2979299505 modified "2023-10-16" @default.
- W2979299505 title "Fused N‐Heterocycles with Contiguous Stereogenic Centers Accessed by an Asymmetric Catalytic Cascade Reaction of Tertiary Enamides" @default.
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- W2979299505 doi "https://doi.org/10.1002/chem.201904596" @default.
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