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- W2979331330 endingPage "18413" @default.
- W2979331330 startingPage "18410" @default.
- W2979331330 abstract "Abstract An N‐heterocyclic carbene (NHC)‐catalyzed reaction between α‐bromoenals and 2‐aminoaldehydes has been developed. Key steps include chemoselective reaction of the NHC catalyst with one of the aldehyde substrates (the bromoenal) to eventually generate an α,β‐unsaturated acylazolium intermediate. Addition of the nitrogen atom of aminoaldehyde to the unsaturated azolium ester intermediate followed by intramolecular aldol reaction, β‐lactone formation, and decarboxylation leads to chiral dihydroquinolines with high optical purity. The dihydroquinoline products, which are quickly prepared by using this method, can be readily transformed into a diverse set of functional molecules such as pyridines and chiral piperidines." @default.
- W2979331330 created "2019-10-18" @default.
- W2979331330 creator A5005455559 @default.
- W2979331330 creator A5018344628 @default.
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- W2979331330 creator A5068733979 @default.
- W2979331330 creator A5086969342 @default.
- W2979331330 creator A5090083650 @default.
- W2979331330 date "2019-11-04" @default.
- W2979331330 modified "2023-10-12" @default.
- W2979331330 title "NHC‐Catalyzed Chemoselective Reactions of Enals and Aminobenzaldehydes for Access to Chiral Dihydroquinolines" @default.
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- W2979331330 doi "https://doi.org/10.1002/anie.201909479" @default.
- W2979331330 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31604001" @default.
- W2979331330 hasPublicationYear "2019" @default.
- W2979331330 type Work @default.